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Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization, and Orientation
Wang, HF (Wang, Hong-Fei); Velarde, L (Velarde, Luis); Gan, W (Gan, Wei); Fu, L (Fu, Li)
2015
发表期刊ANNUAL REVIEW OF PHYSICAL CHEMISTRY
卷号66期号:4页码:189-216
摘要

Sum-frequency generation vibrational spectroscopy (SFG-VS) can provide detailed information and understanding of the molecular composition, interactions, and orientational and conformational structure of surfaces and interfaces through quantitative measurement and analysis. In this review, we present the current status of and discuss important recent developments in the measurement of intrinsic SFG spectral lineshapes and formulations for polarization measurements and orientational analysis of SFG-VS spectra. The focus of this review is to present a coherent description of SFG-VS and discuss the main concepts and issues that can help advance this technique as a quantitative analytical research tool for revealing the chemistry and physics of complex molecular surfaces and interfaces.

关键词Nonlinear Susceptibilities Molecular Polarizability Euler Transformation Interference Fresnel Factor Local Field Factor
DOI10.1146/annurev-physchem-040214-121322
收录类别SCI
WOS记录号WOS:000352259800009
引用统计
文献类型期刊论文
条目标识符http://ir.xjipc.cas.cn/handle/365002/5172
专题环境科学与技术研究室
作者单位1.Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA
2.SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA
3.Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Xinjiang, Peoples R China
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Wang, HF ,Velarde, L ,Gan, W ,et al. Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization, and Orientation[J]. ANNUAL REVIEW OF PHYSICAL CHEMISTRY,2015,66(4):189-216.
APA Wang, HF ,Velarde, L ,Gan, W ,&Fu, L .(2015).Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization, and Orientation.ANNUAL REVIEW OF PHYSICAL CHEMISTRY,66(4),189-216.
MLA Wang, HF ,et al."Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization, and Orientation".ANNUAL REVIEW OF PHYSICAL CHEMISTRY 66.4(2015):189-216.
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