Linear and nonlinear optical properties of aluminum borate crystal Al5BO9: Experiment and calculation
An, DH (An, Donghai); Zhang, M (Zhang, Min); Li, DN (Li, Danni); Pan, SL (Pan, Shilie); Chen, HM (Chen, Huimin); Yang, ZH (Yang, Zhihua); Zhu, YT (Zhu, Yingtao); Sun, Y (Sun, Yi); Zhang, H (Zhang, Hui); Li, YY (Li, Yangyang)
2015
Source PublicationJOURNAL OF MATERIALS RESEARCH
ISSN0884-2914
Volume30Issue:15Pages:2319-2326
Abstract

A noncentrosymmetric aluminum borate crystal, Al5BO9, was obtained via high-temperature solution method. Considering the structure diversities of Al5BO9, the single crystal structure was cautiously redetermined before the investigation. The fundamental building blocks of the structure are BO3 triangles, AlO4 tetrahedra, and AlO6 octahedra. Since Al5BO9 only consists of strong covalent B-O and Al-O bonds, it is worth investigating the structure-optical property relationship thoroughly, especially the linear and nonlinear optical properties. To gain further insight into the origin of the nonlinear optical response of Al5BO9, the electronic structure calculations, second harmonic generation (SHG)-weighted electron density, and dipole moment of polyhedra were analyzed in detail. All evidences deduced from calculated results indicate that the SHG contribution from the Al-O polyhedra is more pronounced than that of the BO3 group in Al5BO9, which is anticipated to open a window for the search and design of new inorganic materials.

DOI10.1557/jmr.2015.204
Indexed BySCI
WOS IDWOS:000359718800006
Citation statistics
Cited Times:4[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.xjipc.cas.cn/handle/365002/5146
Collection中国科学院特殊环境功能材料与器件重点试验室
材料物理与化学研究室
Corresponding AuthorZhang, M (Zhang, Min)
Affiliation1.Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Xinjiang Key Lab Elect Informat Mat & Devices, Key Lab Funct Mat & Devices Special Environm, Urumqi 830011, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
An, DH ,Zhang, M ,Li, DN ,et al. Linear and nonlinear optical properties of aluminum borate crystal Al5BO9: Experiment and calculation[J]. JOURNAL OF MATERIALS RESEARCH,2015,30(15):2319-2326.
APA An, DH .,Zhang, M .,Li, DN .,Pan, SL .,Chen, HM .,...&Li, YY .(2015).Linear and nonlinear optical properties of aluminum borate crystal Al5BO9: Experiment and calculation.JOURNAL OF MATERIALS RESEARCH,30(15),2319-2326.
MLA An, DH ,et al."Linear and nonlinear optical properties of aluminum borate crystal Al5BO9: Experiment and calculation".JOURNAL OF MATERIALS RESEARCH 30.15(2015):2319-2326.
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