The Next-Generation of Nonlinear Optical Materials: Rb3Ba3Li2Al4B6O20F-Synthesis, Characterization, and Crystal Growth
Yu, HW (Yu, Hongwei); Young, J (Young, Joshua); Wu, HP (Wu, Hongping); Zhang, WG (Zhang, Weiguo); Rondinelli, JM (Rondinelli, James M.); Halasyamani, S (Halasyamani, Shiv)
2017
Source PublicationADVANCED OPTICAL MATERIALS
Volume5Issue:23
Abstract

Nonlinear optical (NLO) materials are of intense academic and technological interest attributable to their ability to generate coherent radiation over a range of different wavelengths. The requirements for a viable NLO material are rather strict, and their discovery has mainly been serendipitous. This study reports synthesis, characterization, and, most importantly, growth of large single crystals of a technologically viable NLO material-Rb3Ba3Li2Al4B6O20F. Through the judicious selection of cations, Rb3Ba3Li2Al4B6O20F exhibits a 3D structure that facilitates the growth of large single crystals along the optical axis direction. Measurements on these crystals indicate that Rb3Ba3Li2Al4B6O20F exhibits a moderate birefringence of 0.057 at 1064 nm enabling Type I phase-matching down to 243 nm. Theoretical calculations indicate the symmetry adapted mode displacement (SAMD) parameter scales with the second-harmonic generation intensity.

KeywordBorates Deep-uv Nonlinear Optical Materials Rb3ba3li2al4b6o20f Second-harmonic Generation
DOI10.1002/adom.201700840
Indexed BySCI
WOS IDWOS:000416832000015
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Document Type期刊论文
Identifierhttp://ir.xjipc.cas.cn/handle/365002/5054
Collection中国科学院特殊环境功能材料与器件重点试验室
Affiliation1.Univ Houston, Dept Chem, 112 Fleming Bldg, Houston, TX 77204 USA
2.Naval Res Lab, 4555 Overlook Ave SW, Washington, DC 20375 USA
3.Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, 40-1 Beijing Rd, Urumqi 830011, Xinjiang, Peoples R China
4.Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA
Recommended Citation
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Yu, HW ,Young, J ,Wu, HP ,et al. The Next-Generation of Nonlinear Optical Materials: Rb3Ba3Li2Al4B6O20F-Synthesis, Characterization, and Crystal Growth[J]. ADVANCED OPTICAL MATERIALS,2017,5(23).
APA Yu, HW ,Young, J ,Wu, HP ,Zhang, WG ,Rondinelli, JM ,&Halasyamani, S .(2017).The Next-Generation of Nonlinear Optical Materials: Rb3Ba3Li2Al4B6O20F-Synthesis, Characterization, and Crystal Growth.ADVANCED OPTICAL MATERIALS,5(23).
MLA Yu, HW ,et al."The Next-Generation of Nonlinear Optical Materials: Rb3Ba3Li2Al4B6O20F-Synthesis, Characterization, and Crystal Growth".ADVANCED OPTICAL MATERIALS 5.23(2017).
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