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Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst
Zhang, RH (Zhang, Ronghui); Ma, YB (Ma, Yubo); You, F (You, Feng); Peng, T (Peng, Tao); He, ZC (He, Zhaocheng); Li, KN (Li, Kening)
2017
Source PublicationINTERNATIONAL JOURNAL OF HYDROGEN ENERGY
Volume42Issue:40Pages:25185-25194
Abstract

A cheap and magnetic Ni/Cu/Al/Fe catalyst for the selective hydrogenation of LA into GVL catalysts was prepared by sol-gel method. The reaction pathway was systematically studied by examining the reaction conditions, such as reaction pressure, catalyst loadings, water content, and reaction temperature. Higher reaction pressure and catalyst loadings were prior to form HA, then MHV, finally GVL; ML was easily to form with a higher reaction temperature. Water, as a key role, which was in favor to form HA, then MHV, finally GVL; more important, a higher LA conversion could be obtained in methanol as the solvent with some certain content of water. And, it can give a reference for future new clean energy vehicles' application. (C) 2017 Hydrogen Energy Publications LLC.

KeywordLevulinic Acid Gamma-valerolactone Methyl Levulinate Reaction Pathway Hydrogenation Future Clean-energy Vehicles
DOI10.1016/j.ijhydene.2017.08.121
Indexed BySCI
WOS IDWOS:000413284500005
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Document Type期刊论文
Identifierhttp://ir.xjipc.cas.cn/handle/365002/5033
Collection资源化学研究室
Affiliation1.Sun Yat Sen Univ, Sch Engn, Guangdong Key Lab Intelligent Transportat Syst, Guangzhou 510275, Guangdong, Peoples R China
2.Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Xinjiang, Peoples R China
3.South China Univ Technol, Sch Civil Engn & Transportat, Guangzhou 510640, Guangdong, Peoples R China
4.Tianjin Univ Technol & Educ, Coll Automobile & Transportat, Tianjin 300222, Peoples R China
5.Shanghai Jiao Tong Univ, State Key Lab Mech Syst & Vibrat, Shanghai 200240, Peoples R China
Recommended Citation
GB/T 7714
Zhang, RH ,Ma, YB ,You, F ,et al. Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2017,42(40):25185-25194.
APA Zhang, RH ,Ma, YB ,You, F ,Peng, T ,He, ZC ,&Li, KN .(2017).Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,42(40),25185-25194.
MLA Zhang, RH ,et al."Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 42.40(2017):25185-25194.
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