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Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst
Zhang, RH (Zhang, Ronghui); Ma, YB (Ma, Yubo); You, F (You, Feng); Peng, T (Peng, Tao); He, ZC (He, Zhaocheng); Li, KN (Li, Kening)
2017
发表期刊INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷号42期号:40页码:25185-25194
摘要

A cheap and magnetic Ni/Cu/Al/Fe catalyst for the selective hydrogenation of LA into GVL catalysts was prepared by sol-gel method. The reaction pathway was systematically studied by examining the reaction conditions, such as reaction pressure, catalyst loadings, water content, and reaction temperature. Higher reaction pressure and catalyst loadings were prior to form HA, then MHV, finally GVL; ML was easily to form with a higher reaction temperature. Water, as a key role, which was in favor to form HA, then MHV, finally GVL; more important, a higher LA conversion could be obtained in methanol as the solvent with some certain content of water. And, it can give a reference for future new clean energy vehicles' application. (C) 2017 Hydrogen Energy Publications LLC.

关键词Levulinic Acid Gamma-valerolactone Methyl Levulinate Reaction Pathway Hydrogenation Future Clean-energy Vehicles
DOI10.1016/j.ijhydene.2017.08.121
收录类别SCI
WOS记录号WOS:000413284500005
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.xjipc.cas.cn/handle/365002/5033
专题资源化学研究室
作者单位1.Sun Yat Sen Univ, Sch Engn, Guangdong Key Lab Intelligent Transportat Syst, Guangzhou 510275, Guangdong, Peoples R China
2.Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Xinjiang, Peoples R China
3.South China Univ Technol, Sch Civil Engn & Transportat, Guangzhou 510640, Guangdong, Peoples R China
4.Tianjin Univ Technol & Educ, Coll Automobile & Transportat, Tianjin 300222, Peoples R China
5.Shanghai Jiao Tong Univ, State Key Lab Mech Syst & Vibrat, Shanghai 200240, Peoples R China
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Zhang, RH ,Ma, YB ,You, F ,et al. Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2017,42(40):25185-25194.
APA Zhang, RH ,Ma, YB ,You, F ,Peng, T ,He, ZC ,&Li, KN .(2017).Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,42(40),25185-25194.
MLA Zhang, RH ,et al."Exploring to direct the reaction pathway for hydrogenation of levulinic acid into gamma-valerolactone for future Clean-Energy Vehicles over a magnetic Cu-Ni catalyst".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 42.40(2017):25185-25194.
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