New Compressed Chalcopyrite-like Li(2)BaM(IV)Q(4) (M-IV = Ge, Sn; Q = S, Se): Promising Infrared Nonlinear Optical Materials
Wu, K (Wu, Kui); Zhang, BB (Zhang, Bingbing); Yang, ZH (Yang, Zhihua); Pan, SL (Pan, Shilie); Yang, ZH; Pan, SL
2017
发表期刊JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷号139期号:42页码:14885-14888
摘要

Chalcopyrite-type AgGaQ(2) (Q = S, Se) and ZnGeP2 are the main commercial infrared nonlinear optical (IR NLO) crystals. Unfortunately, performance defects including low laser damage threshold (LDT), harmful two-photon absorption (TPA), or small birefringence limit their application. With this background, four new compressed chalcopyrite-like IR NLO materials Li(2)BaM(IV)Q(4) (M-IV = Ge, Sn; Q= S, Se) were successfully synthesized with the typical AgGaQ2 as templates. Remarkably, Li2BaGeS4 and Li2BaSnS4 not only maintain the good NLO responses (0.5 and 0.7 X AgGaS2) but also overcome low LDTs and TPA of commercial chalcopyrites, demonstrating that they satisfy critical demands as promising IR NLO candidates. All of them exhibit phase matching abilities. Furthermore, the discovery of chalcopyrite-like compounds also provides a feasible design strategy to explore new promising IR NLO materials.

DOI10.1021/jacs.7b08966
收录类别SCI
WOS记录号WOS:000414115800017
引用统计
被引频次:18[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.xjipc.cas.cn/handle/365002/5029
专题中国科学院特殊环境功能材料与器件重点试验室
通讯作者Yang, ZH; Pan, SL
作者单位Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Key Lab Funct Mat & Devices Special Environm, Xinjiang Key Lab Elect Informat Mat & Devices, 40-1 South Beijing Rd, Urumqi 830011, Peoples R China
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Wu, K ,Zhang, BB ,Yang, ZH ,et al. New Compressed Chalcopyrite-like Li(2)BaM(IV)Q(4) (M-IV = Ge, Sn; Q = S, Se): Promising Infrared Nonlinear Optical Materials[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2017,139(42):14885-14888.
APA Wu, K ,Zhang, BB ,Yang, ZH ,Pan, SL ,Yang, ZH,&Pan, SL.(2017).New Compressed Chalcopyrite-like Li(2)BaM(IV)Q(4) (M-IV = Ge, Sn; Q = S, Se): Promising Infrared Nonlinear Optical Materials.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,139(42),14885-14888.
MLA Wu, K ,et al."New Compressed Chalcopyrite-like Li(2)BaM(IV)Q(4) (M-IV = Ge, Sn; Q = S, Se): Promising Infrared Nonlinear Optical Materials".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 139.42(2017):14885-14888.
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