CsB4O6F: ACongruent-Melting Deep-Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units
Wang, XF (Wang, Xuefei)[ 1,2 ]; Wang, Y (Wang, Ying)[ 1 ]; Zhang, BB (Zhang, Bingbing)[ 1 ]; Zhang, FF (Zhang, Fangfang)[ 1 ]; Yang, ZH (Yang, Zhihua)[ 1 ]; Pan, SL (Pan, Shilie)[ 1 ]
2017
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
ISSN1433-7851
Volume56Issue:45Pages:14119-14123
Abstract

The discovery of new nonlinear optical (NLO) materials for coherent light generation in the deep-ultraviolet (DUV, wavelength below 200 nm) region is essential for the development of laser technologies. Herein, we report a new material CsB4O6F (CBF), which combines the superior structural properties of two well-known NLO materials, beta-BaB2O4 (BBO) and KBe2BO3F2 (KBBF). CBF exhibits excellent DUV optical properties including a short cutoff edge (155 nm), a large SHG response (approximate to 1.9 X KDP), and a suitable birefringence that enables frequency doubling down to 171.6 nm. Remarkably, CBF melts congruently and shows an improved growth habit. In addition, our rational design strategy will contribute to the discovery of DUV NLO materials.

KeywordDeep-ultraviolet Fluorooxoborates Nonlinear Optical Materials Second Harmonic Generation
DOI10.1002/ange.201708231
Indexed BySCI
WOS IDWOS:000413896400036
Citation statistics
Cited Times:102[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.xjipc.cas.cn/handle/365002/5023
Collection中国科学院特殊环境功能材料与器件重点试验室
材料物理与化学研究室
Corresponding AuthorWang, Y (Wang, Ying)[ 1 ]; Zhang, FF (Zhang, Fangfang)[ 1 ]; Pan, SL (Pan, Shilie)[ 1 ]
AffiliationChinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Xinjiang Key Lab Elect Informat Mat & Devices, Key Lab Funct Mat & Devices Special Environm, 40-1 South Beijing Rd, Urumqi 830011, Peoples R China;Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Wang, XF ,Wang, Y ,Zhang, BB ,et al. CsB4O6F: ACongruent-Melting Deep-Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2017,56(45):14119-14123.
APA Wang, XF ,Wang, Y ,Zhang, BB ,Zhang, FF ,Yang, ZH ,&Pan, SL .(2017).CsB4O6F: ACongruent-Melting Deep-Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,56(45),14119-14123.
MLA Wang, XF ,et al."CsB4O6F: ACongruent-Melting Deep-Ultraviolet Nonlinear Optical Material by Combining Superior Functional Units".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 56.45(2017):14119-14123.
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