Evidence of "new hot spots'' from determining the nonlinear optical behavior of materials: mechanistic studies of the vanadium borate crystal, Na3VO2B6O11
Su, X (Su, Xin); Yang, ZH (Yang, Zhihua); Lee, MH (Lee, Ming-Hsien); Pan, SL (Pan, Shilie); Wang, Y (Wang, Ying); Fan, XY (Fan, Xiaoyun); Huang, ZJ (Huang, Zhenjun); Zhang, BB (Zhang, Bingbing); Yang, ZH
2015
发表期刊PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷号17期号:7页码:5338-5344
摘要A novel mechanism for the nonlinear optical (NLO) effects of vanadium borate crystals, Na3VO2B6O11 (NVB), with distorted VO4 groups was investigated. A comprehensive analysis of the structure-property relationship was performed by combining the experimental measurements, the electronic structures calculations, the SHG-weighted electron density and the real-space atom-contribution analysis to yield the linear and nonlinear optical properties. The contribution of a (VO4)(3-) anionic group to the second harmonic generation (SHG) response was more pronounced than that of the (BO3)(3-) anionic group, which plays a virtual role in the SHG effects in NVB. The anionic (BO3)(3-) groups make dominant contributions to the birefringence, whereas the contribution of the V5+ cations to these linear optical effects is negligible.
DOI10.1039/c4cp04248d
收录类别SCI
WOS记录号WOS:000349616400062
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文献类型期刊论文
条目标识符http://ir.xjipc.cas.cn/handle/365002/4862
专题中国科学院特殊环境功能材料与器件重点试验室
材料物理与化学研究室
通讯作者Yang, ZH
作者单位1.Chinese Acad Sci, Key Lab Funct Mat & Devices Special Environm, Xinjiang Key Lab Elect Informat Mat & Devices, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Tamkang Univ, Dept Phys, Taipei 25137, Taiwan
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Su, X ,Yang, ZH ,Lee, MH ,et al. Evidence of "new hot spots'' from determining the nonlinear optical behavior of materials: mechanistic studies of the vanadium borate crystal, Na3VO2B6O11[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2015,17(7):5338-5344.
APA Su, X .,Yang, ZH .,Lee, MH .,Pan, SL .,Wang, Y .,...&Yang, ZH.(2015).Evidence of "new hot spots'' from determining the nonlinear optical behavior of materials: mechanistic studies of the vanadium borate crystal, Na3VO2B6O11.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,17(7),5338-5344.
MLA Su, X ,et al."Evidence of "new hot spots'' from determining the nonlinear optical behavior of materials: mechanistic studies of the vanadium borate crystal, Na3VO2B6O11".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 17.7(2015):5338-5344.
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