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Cross-Propagation Sum-Frequency Generation Vibrational Spectroscopy
Fu, L (Fu, Li); Chen, SL (Chen, Shun-li); Gan, W (Gan, Wei); Wang, HF (Wang, Hong-fei)

Here we report the theory formulation and the experiment realization of sum-frequency generation vibrational spectroscopy (SFG-VS) in the cross-propagation (XP) geometry or configuration. In the XP-SFG-VS, the visible and the infrared (IR) beams in the SFG experiment are delivered to the same location on the surface from visible and IR incident planes perpendicular to each other, avoiding the requirement to have windows or optics to be transparent to both the visible and IR frequencies. Therefore, the XP geometry is applicable to study surfaces in the enclosed vacuum or high pressure chambers with far infrared (FIR) frequencies that can directly access the metal oxide and other lower frequency surface modes, with much broader selection of visible and IR transparent window materials. The potential applications include surface science, material science, fundamental catalytic sciences, as well as low temperature molecular sciences, etc.

KeywordSum-frequency Generation Vibrational Spectroscopy Co-propagation Counter-propagation Cross-propagation
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WOS IDWOS:000373211400009
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Cited Times:3[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Affiliation1.Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA
2.Chinese Acad Sci, Xinjiang Tech Inst Phys Chem, Lab Environm Sci & Technol, Key Lab Funct Mat & Devices Special Environm, Urumqi 830011, Peoples R China
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GB/T 7714
Fu, L ,Chen, SL ,Gan, W ,et al. Cross-Propagation Sum-Frequency Generation Vibrational Spectroscopy[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2016,29(1):70-80.
APA Fu, L ,Chen, SL ,Gan, W ,&Wang, HF .(2016).Cross-Propagation Sum-Frequency Generation Vibrational Spectroscopy.CHINESE JOURNAL OF CHEMICAL PHYSICS,29(1),70-80.
MLA Fu, L ,et al."Cross-Propagation Sum-Frequency Generation Vibrational Spectroscopy".CHINESE JOURNAL OF CHEMICAL PHYSICS 29.1(2016):70-80.
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