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One-Pot Synthesis of Graphene-Supported Monodisperse Pd Nanoparticles as Catalyst for Formic Acid Electro-oxidation
Yang, Sudong; Dong, Jing; Yao, Zhaohui; Shen, Chengmin; Shi, Xuezhao; Tian, Yuan; Lin, Shaoxiong; Zhang, Xiaogang
2014
发表期刊SCIENTIFIC REPORTS
ISSN2045-2322
卷号4期号:3
摘要To synthesize monodisperse palladium nanoparticles dispersed on reduced graphene oxide (RGO) sheets, we have developed an easy and scalable solvothermal reduction method from an organic solution system. The RGO-supported palladium nanoparticles with a diameter of 3.8 nm are synthesized in N-methyl-2-pyrrolidone (NMP) and in the presence of oleylamine and trioctylphosphine, which facilitates simultaneous reduction of graphene oxide and formation of Pd nanocrystals. So-produced Pd/RGO was tested for potential use as electrocatalyst for the electro-oxidation of formic acid. Pd/RGO catalyzes formic acid oxidation very well compared to Pd/Vulcan XC-72 catalyst. This synthesis method is a new way to prepare excellent electrocatalysts, which is of great significance in energy-related catalysis.
DOI10.1038/srep04501
收录类别SCI
WOS记录号WOS:000333515700008
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被引频次:73[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.xjipc.cas.cn/handle/365002/3797
专题环境科学与技术研究室
作者单位Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China;Tsinghua Univ, Sch Aerosp, Beijing 100084, Peoples R China;Nanjing Univ Aeronaut & Astronaut, Coll Mat Sci & Engn, Nanjing 210016, Peoples R China;Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Lab Ecomat & Sustainable Technol LEMST, Urumqi 830011, Peoples R China
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Yang, Sudong,Dong, Jing,Yao, Zhaohui,et al. One-Pot Synthesis of Graphene-Supported Monodisperse Pd Nanoparticles as Catalyst for Formic Acid Electro-oxidation[J]. SCIENTIFIC REPORTS,2014,4(3).
APA Yang, Sudong.,Dong, Jing.,Yao, Zhaohui.,Shen, Chengmin.,Shi, Xuezhao.,...&Zhang, Xiaogang.(2014).One-Pot Synthesis of Graphene-Supported Monodisperse Pd Nanoparticles as Catalyst for Formic Acid Electro-oxidation.SCIENTIFIC REPORTS,4(3).
MLA Yang, Sudong,et al."One-Pot Synthesis of Graphene-Supported Monodisperse Pd Nanoparticles as Catalyst for Formic Acid Electro-oxidation".SCIENTIFIC REPORTS 4.3(2014).
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