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Electrosynthesis of poly(3,4-ethylenedithiathiophene) in an ionic liquid and its electrochemistry and electrochromic properties
Lu Baoyang; Zhang Shimin; Qin Leiqiang; Chen Shuai; Zhen Shijie; Xu Jingkun
2013
发表期刊ELECTROCHIMICA ACTA
ISSN0013-4686
卷号106期号:9页码:201-208
摘要We herein report the electrosynthesis of the all-sulfur analog of PEDOT, poly(3,4-ethylenedithiathiophene) (PEDTT), in air and moisture stable ionic liquid 1-butyl-3-methylimidazolium hexafluorophosphate (BmimPF(6)). The as-obtained PEDTT film was studied by FT-IR, SEM, GPC, UV-vis spectroscopy, fluorescence and thermal analysis, respectively. Electrochemistry results demonstrated that PEDTT film could be further doped by cyclic voltammetry to substantially improve its doping level. Besides, PEDTT exhibits electrochromic nature with its color changing from golden brown in its reduced form to grass green upon oxidation. By further investigation, PEDTT was also found to reveal favorable coloration efficiency of 127 cm(2) C-1 comparable to PEDOT, low switching voltages and favorable electroactivity and stability. (c) 2013 Elsevier Ltd. All rights reserved.
关键词Electropolymerization Poly(3 Ionic Liquids 4-ethylenedithiathiophene) Redoping Electrochromics
学科领域Electrochemistry
DOI10.1016/j.electacta.2013.05.068
收录类别SCI
WOS记录号WOS:000323192400026
引用统计
文献类型期刊论文
条目标识符http://ir.xjipc.cas.cn/handle/365002/2634
专题环境科学与技术研究室
作者单位Jiangxi Sci & Technol Normal Univ, Sch Pharm, Nanchang 330013, Peoples R China;Shandong Univ, Sch Mat Sci & Engn, Jinan 250061, Peoples R China;Chinese Acad Sci, Lab Environm Sci & Technol, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Peoples R China
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Lu Baoyang,Zhang Shimin,Qin Leiqiang,et al. Electrosynthesis of poly(3,4-ethylenedithiathiophene) in an ionic liquid and its electrochemistry and electrochromic properties[J]. ELECTROCHIMICA ACTA,2013,106(9):201-208.
APA Lu Baoyang,Zhang Shimin,Qin Leiqiang,Chen Shuai,Zhen Shijie,&Xu Jingkun.(2013).Electrosynthesis of poly(3,4-ethylenedithiathiophene) in an ionic liquid and its electrochemistry and electrochromic properties.ELECTROCHIMICA ACTA,106(9),201-208.
MLA Lu Baoyang,et al."Electrosynthesis of poly(3,4-ethylenedithiathiophene) in an ionic liquid and its electrochemistry and electrochromic properties".ELECTROCHIMICA ACTA 106.9(2013):201-208.
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