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TiO2 supported on silica nanolayers derived from vermiculite for efficient photocatalysis
Wang Lan; Wang Xu; Cui Sifang; Fan Xiaoyun; Zu Baiyi; Wang Chuanyi
2013
发表期刊CATALYSIS TODAY
ISSN0920-5861
卷号216期号:11页码:95-103
摘要Various TiO2 composite photocatalysts were synthesized by immobilizing TiO2 nanoparticles onto the surface of silica nanolayers (SNLs) derived from vermiculite via a simple reaction between titanium hydrate and SNLs by varying Ti/SNLs ratios and using different acidic media (HCl, HNO3 and H2SO4). As-obtained composites were characterized by means of XRD, SEM and BET analytical techniques. The photocatalytic activities of photocatalysts were evaluated using methylene blue (MB) as a model pollutantin aqueous solution. It was found that the acidic media HCl and HNO3 favored the formation of tri-crystalline and flat spongy-like thin layers of TiO2 nanoparticles with large specific surface area giving excellent photocatalytic activity; while H2SO4 medium resulted in the single-phase of anatase TiO2 with ball-like aggregates on the TiO2 thin layer, giving relatively low photocatalytic activity. The excellent performance of the composites obtained using proper SNLs content and suitable acidic medium can be mainly ascribed to the mixed-phase structures with an optimum ratio and large specific surface area, as well as the facile immobilization of TiO2 on the support, which will be beneficial to their separation from water treatment system in practical application.
关键词Tio2 Immobilization Silica Nanolayers Vermiculite Different Acids Photocatalysis
学科领域Chemistry ; Engineering
DOI10.1016/j.cattod.2013.06.026
收录类别SCI
WOS记录号WOS:000324296400016
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.xjipc.cas.cn/handle/365002/2629
专题环境科学与技术研究室
作者单位Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Lab Environm Sci & Technol, Key Lab Funct Mat & Devices Special Environm, Urumqi 830011, Peoples R China;Chinese Acad Sci, Xinjiang Tech Inst Phys & Chem, Lab Green Chem & Organ Synth, Urumqi 830011, Peoples R China; Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, Wuhan 430074, Peoples R China
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GB/T 7714
Wang Lan,Wang Xu,Cui Sifang,et al. TiO2 supported on silica nanolayers derived from vermiculite for efficient photocatalysis[J]. CATALYSIS TODAY,2013,216(11):95-103.
APA Wang Lan,Wang Xu,Cui Sifang,Fan Xiaoyun,Zu Baiyi,&Wang Chuanyi.(2013).TiO2 supported on silica nanolayers derived from vermiculite for efficient photocatalysis.CATALYSIS TODAY,216(11),95-103.
MLA Wang Lan,et al."TiO2 supported on silica nanolayers derived from vermiculite for efficient photocatalysis".CATALYSIS TODAY 216.11(2013):95-103.
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