BaClBF4: a new noncentrosymmetric pseudo-Aurivillius type material with transparency range from deep UV to middle IR and a high laser damage threshold
Zhang, M (Zhang, Min)[ 1 ]; Pan, SL (Pan, Shilie)[ 1 ]; Yang, ZH (Yang, Zhihua)[ 1 ]; Wang, Y (Wang, Ying)[ 1,2 ]; Su, X (Su, Xin)[ 1,2 ]; Yang, Y (Yang, Yun)[ 1 ]; Huang, ZJ (Huang, Zhenjun)[ 1,2 ]; Han, SJ (Han, Shujuan)[ 1 ]; Poeppelmeier, KR (Poeppelmeier, Kenneth R.)[ 3 ]
2013
Source PublicationJournal of Materials Chemistry C
ISSN2050-7526
Volume1Issue:31Pages:4740-4745
Abstract

A new noncentrosymmetric alkaline earth metal halide borate, BaClBF4, has been synthesized with crystal size up to 6 mm x 6 mm x 3 mm via the hydrothermal method at 200 degrees C. The crystal structure can be described as an alternate stacking of cationic [Ba2Cl2](2+) layers with anionic [BF4](-) layers along the b direction, and the [Ba2Cl2](2+) layer is a pseudo-Aurivillius type layer similar to the [Bi2O2](2+) layer. The transmittance range of BaClBF4 is from 0.18 to 8.5 mu m, and the laser damage threshold of the crystal is about 6.8 GW cm(-2). EDS, TG-DSC and second harmonic generation investigations are reported. The electronic structure is discussed to explain the structure-property relationships.

DOI10.1039/c3tc30581c
Indexed BySCI
WOS IDWOS:000322028700017
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Cited Times:23[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.xjipc.cas.cn/handle/365002/2549
Collection新疆维吾尔自治区电子信息材料与器件重点实验室
材料物理与化学研究室
Corresponding AuthorPan, SL (Pan, Shilie)[ 1 ]
Affiliation1.Chinese Acad Sci, Xinjiang Key Lab Elect Informat Mat & Devices, Key Lab Funct Mat & Devices Special Environm, Xinjiang Tech Inst Phys & Chem, Urumqi 830011, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Northwestern Univ, Dept Chem, Evanston, IL 60208 USA
Recommended Citation
GB/T 7714
Zhang, M ,Pan, SL ,Yang, ZH ,et al. BaClBF4: a new noncentrosymmetric pseudo-Aurivillius type material with transparency range from deep UV to middle IR and a high laser damage threshold[J]. Journal of Materials Chemistry C,2013,1(31):4740-4745.
APA Zhang, M .,Pan, SL .,Yang, ZH .,Wang, Y .,Su, X .,...&Poeppelmeier, KR .(2013).BaClBF4: a new noncentrosymmetric pseudo-Aurivillius type material with transparency range from deep UV to middle IR and a high laser damage threshold.Journal of Materials Chemistry C,1(31),4740-4745.
MLA Zhang, M ,et al."BaClBF4: a new noncentrosymmetric pseudo-Aurivillius type material with transparency range from deep UV to middle IR and a high laser damage threshold".Journal of Materials Chemistry C 1.31(2013):4740-4745.
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